Two-color spin noise spectroscopy: Using spin fluctuation correlations to reveal homogeneous linewidths within quantum dot ensembles

TL;DR

This paper introduces a two-color spin noise spectroscopy method that uses spin fluctuation correlations to measure homogeneous linewidths within quantum dot ensembles, surpassing limitations of traditional spectroscopy.

Contribution

It demonstrates a novel noise correlation technique that reveals homogeneous linewidths in inhomogeneously broadened systems using two weak probe lasers.

Findings

Correlation of spin noise signals depends on laser detuning

Homogeneous linewidths can be extracted from noise correlations

Method applicable to various systems with measurable intrinsic fluctuations

Abstract

"Spin noise spectroscopy" (SNS) is a powerful optical technique for probing electron and hole spin dynamics that is based on detecting their intrinsic and random fluctuations while in thermal equilibrium, an approach guaranteed by the fluctuation-dissipation theorem. Because SNS measures fluctuation properties rather than conventional response functions, we show that fluctuation \emph{correlations} can be exploited in multi-probe noise studies to reveal information that in general cannot be accessed by conventional linear optical spectroscopy, such as the underlying homogeneous linewidths of individual constituents within inhomogeneously-broadened systems. This is demonstrated in an ensemble of singly-charged (In,Ga)As quantum dots using two weak probe lasers: When the two lasers have the same wavelength, they are sensitive to the same QDs in the ensemble and their spin fluctuation signals are correlated. In contrast, two probe lasers that are widely detuned from each other measure different subsets of QDs, leading to uncorrelated fluctuations. Measuring the noise correlation versus laser detuning directly reveals the QD homogeneous linewidth even in the presence of a strong inhomogeneous broadening. Such noise-based correlation techniques are not limited to semiconductor spin systems, but can be widely applied to any system in which intrinsic fluctuations are measurable.