High-Energy Damping by Particle-Hole Excitations in the Spin-Wave Spectrum of Iron-Based Superconductors

TL;DR

This paper models the spin excitation spectra of iron pnictides using a double-exchange model, revealing how itinerant electrons influence high-energy spin-wave damping and aligning with neutron scattering observations.

Contribution

It introduces a fermionic spinon approach combined with RPA calculations to analyze spin excitations in iron-based superconductors, highlighting the role of itinerant electrons in damping high-energy spin waves.

Findings

Spin-wave excitation at (π,π) is elevated in energy due to itinerant electrons.

Particle-hole continuum maintains high-energy spin excitations without C4 symmetry breaking.

Results are consistent with recent neutron scattering experiments.

Abstract

Using a degenerate double-exchange model, we investigate the spin excitation spectra of iron pnictides. The model consists of local spin moments on each Fe site, as well as itinerant electrons from the degenerate $d_{xz}$ and $d_{yz}$ orbitals. The local moments interact with each other through antiferromagnetic $J_{1}$-$J_{2}$ Heisenberg interactions, and they couple to the itinerant electrons through a ferromagnetic Hund coupling. We employ the fermionic spinon representation for the local moments and perform a generalized random-phase approximation calculation on both spinons and itinerant electrons. We find that in the $\left(\pi,0\right)$ magnetically-ordered state, the spin-wave excitation at $\left(\pi,\pi\right)$ is pushed to a higher energy due to the presence of itinerant electrons, which is consistent with a previous study using the Holstein-Primakoff transformation. In the paramagnetic state, the particle-hole continuum keeps the collective spin excitation near $\left(\pi,\pi\right)$ at a higher energy even without any $C_{4}$ symmetry breaking. The implications for recent high temperature neutron scattering measurements will be discussed.