Proposed method for laser spectroscopy of pionic helium atoms to determine the charged-pion mass

TL;DR

This paper calculates energy levels, decay rates, and proposes a laser spectroscopy method for metastable pionic helium atoms to precisely determine the charged-pion mass, involving quantum electrodynamics corrections and metastable state manipulations.

Contribution

It introduces a detailed theoretical framework for laser-induced transitions in pionic helium to facilitate precise pion mass measurements, including metastable state identification and decay dynamics.

Findings

Calculated energy levels with relativistic and QED corrections.

Identified metastable states with nanosecond lifetimes.

Proposed laser spectroscopy technique for pion mass determination.

Abstract

Metastable pionic helium ($\pi{\rm He}^+$) is a three-body atom composed of a helium nucleus, an electron occupying the $1s$ ground state, and a negatively charged pion $\pi^-$ in a Rydberg state with principal- and orbital angular momentum quantum numbers of $n\sim \ell+1\sim 16$. We calculate the spin-independent energies of the $\pi{\rm ^3He}^+$ and $\pi{\rm ^4He}^+$ isotopes in the region $n=15$--19. These include relativistic and quantum electrodynamics corrections of orders $R_{\infty}\alpha^2$ and $R_{\infty}\alpha^3$ in atomic units, where $R_{\infty}$ and $\alpha$ denote the Rydberg and fine structure constants. The fine-structure splitting due to the coupling between the electron spin and the orbital angular momentum of the $\pi^-$, and the radiative and Auger decay rates of the states are also calculated. Some states $(n,\ell)=(16,15)$ and $(17,16)$ retain nanosecond-scale lifetimes against $\pi^-$ absorption into the helium nucleus. We propose to use laser pulses to induce $\pi^-$ transitions from these metastable states, to states with large ($\sim 10^{11}$ s$^{-1}$) Auger rates. The $\pi{\rm He}^{2+}$ ion that remains after Auger emission of the $1s$ electron undergoes Stark mixing with the $s$, $p$, and $d$ states during collisions with the helium atoms in the experimental target. This leads to immediate nuclear absorption of the $\pi^-$. The resonance condition between the laser beam and the atom is thus revealed as a sharp spike in the rates of neutrons, protons, deuterons, and tritons that emerge....(continued)