Real-space collapse of a polariton condensate

TL;DR

This paper reports the observation of a real-space collapse of a polariton condensate into a localized peak, suggesting a self-trapping mechanism possibly involving local lattice heating, which challenges conventional understanding of polariton interactions.

Contribution

The study provides the first ultrafast imaging evidence of polariton condensate collapse and proposes a novel self-trapping mechanism involving local heating and polaron formation.

Findings

Observation of condensate collapsing into a localized peak

Ultrafast imaging tracking real and reciprocal space dynamics

Proposed self-trapping via local lattice heating and polaron formation

Abstract

Polaritons in microcavities are versatile quasi-2D bosonic particles with a high degree of coherence and strong nonlinearities, thanks to their hybrid light-matter character. In their condensed form, they display striking quantum hydrodynamic features analogous to atomic Bose-Einstein condensates, such as long-range order coherence, superfluidity and quantized vorticity. Their variegated dispersive and dissipative properties, however, set significant differences from their atomic counterpart. In this work, we report the unique phenomenology that is observed when a pulse of light impacts the polariton vacuum: the condensate that is instantaneously formed does not splash in real space but instead coheres into an enigmatic structure, featuring concentric rings and, most notably, a sharp and bright peak at the center. Using a state-of-the-art ultrafast imaging with 50 fs time steps, we are able to track the dynamics of the polariton mean-field wavefunction in both real and reciprocal space. The observation of the real-space collapse of the condensate into an extremely localized---resolution limited---peak is at odd with the repulsive interactions of polaritons and their positive effective mass. An unconventional mechanism is therefore at play to account for our observations. Our modeling suggests that self-trapping due to a local heating of the crystal lattice---that can be described as a collective polaron formed by a polariton condensate---could be involved. These observations hint at the fascinating fluid dynamics of polaritons in conditions of extreme intensities and ultrafast times.