Electrical and Magnetic behaviour of PrFeAsO0.8F0.2 superconductor

TL;DR

This study synthesizes and characterizes PrFeAsO0.8F0.2 superconductor, revealing its high critical field, critical current density, and suppression of magnetic anomalies seen in the non-superconducting parent compound.

Contribution

It provides detailed electrical and magnetic measurements of PrFeAsO0.8F0.2, demonstrating its superconducting properties and high upper critical field using a simple synthesis method.

Findings

Superconducting transition temperature (Tc) around 38K.

Upper critical field (Hc2) estimated at ~182 Tesla.

Critical current density (Jc) of approximately 10^3 A/cm².

Abstract

The superconducting and ground state samples of PrFeAsO0.8F0.2 and PrFeAsO have been synthesised via easy and versatile single step solid state reaction route. X-ray & Reitveld refine parameters of the synthesised samples are in good agreement to the earlier reported value of the structure. The ground state of the pristine compound (PrFeAsO) exhibited a metallic like step in resistivity below 150K followed by another step at 12K. The former is associated with the spin density wave (SDW) like ordering of Fe spins and later to the anomalous magnetic ordering for Pr moments. Both the resistivity anomalies are absent in case of superconducting PrFeAsO0.8F0.2 sample. Detailed high field (up to 12Tesla) electrical and magnetization measurements are carried out for superconducting PrFeAsO0.8F0.2 sample. The PrFeAsO0.8F0.2 exhibited superconducting onset (Tconset) at around 47K with Tc({\rho} =0) at 38K. Though the Tconset remains nearly invariant, the Tc({\rho} =0) is decreased with applied field, and the same is around 23K under applied field of 12Tesla. The upper critical field (Hc2) is estimated from the Ginzburg Landau equation (GL) fitting, which is found to be ~ 182Tesla. Critical current density (Jc) being calculated from high field isothermal magnetization (MH) loops with the help of Beans critical state model, is found to be of the order of 103 A/cm2. Summarily, the superconductivity characterization of single step synthesised PrFeAsO0.8F0.2 superconductor is presented.