Surface Plasmons and Nonlocality: a Simple Model

TL;DR

This paper introduces a simple local model to simulate nonlocal effects in surface plasmons, enabling easier analysis and computation of atomic-scale light-matter interactions at metal interfaces.

Contribution

A novel local analogue model that replaces nonlocal metals with a composite structure to simplify analysis of nonlocal plasmonic effects.

Findings

The model accurately reproduces nonlocal effects in plasmonic phenomena.

It simplifies numerical simulations of atomic-scale light interactions.

Provides physical insight into nonlocality in plasmonics.

Abstract

Surface plasmons on metals can concentrate light into sub-nanometric volumes and on these near atomic length scales the electronic response at the metal interface is smeared out over a Thomas-Fermi screening length. This nonlocality is a barrier to a good understanding of atomic scale response to light and complicates the practical matter of computing the fields. In this letter, we present a local analogue model and show that spatial nonlocality can be represented by replacing the nonlocal metal with a composite material, comprising a thin dielectric layer on top of a local metal. This method not only makes possible the quantitative analysis of nonlocal effects in complex plasmonic phenomena with unprecedented simplicity and physical insight, but also offers great practical advantages in their numerical treatment.