Revealing quantum path details in high-field physics

TL;DR

This paper introduces a novel method to visualize the phase and amplitude distribution of extreme-ultraviolet radiation generated in strong-field laser-atom interactions, revealing detailed quantum electron dynamics.

Contribution

It presents a phase-sensitive imaging technique based on ion spatial distributions, overcoming previous spatial averaging limitations in EUV measurements.

Findings

Successfully visualized EUV amplitude and phase distributions

Provided new insights into electron wave-packet interference

Enabled phase-controlled interaction studies

Abstract

The tunnelling of an electron through a suppressed atomic potential followed by its motion in the continuum, is the fundamental mechanism underlying strong-field laser-atom/molecule interactions. Due to its quantum nature, the interaction is governed by the phase of the released electron wave-packets. Thus, detailed mapping of the electron wave-packet interferences provides essential insight into the physics underlying the interaction. A process which is providing access to the intricacies of the interaction is the generation of high order harmonics of the laser frequency. The phase-amplitude distribution of the emitted extreme-ultraviolet (EUV), carries the complete information about the harmonic generation process and vice-versa. Thus, the visualization of the EUV-spatial-amplitude-distribution, as it results from interfering electron wave-packet contributions, is of crucial importance. Restrictions to this accomplishment are due to the spatially integrating measurement approaches applied so far, that average out the phase effects in the generation process. In this work, we demonstrate a method which overcomes this obstacle. An EUV-spatial-amplitude-distribution-image is induced from the imprint on the measured spatial distribution of ions, produced through EUV-photon ionization of atoms. Interference extremes in the image carry phase information about the interfering electron wave-packets. The present approach provides detailed insight on the strong-field laser-atom interaction mechanism, while establishing the era of phase selective interaction studies. Furthermore, it paves the way for substantial enhancement of the spectral and temporal precision of measurements by in-situ controlling the phase distribution of the emitted radiation and/or spatially selecting the EUV-radiation-atom interaction products.