Non-linear absorption and density dependent dephasing in Rydberg EIT-media

TL;DR

This paper investigates non-linear light propagation in ultra-cold Rydberg atom ensembles under EIT, revealing density-dependent effects and proposing a Monte Carlo model that aligns with experimental data at low intensities.

Contribution

The authors develop a self-consistent Monte Carlo rate equation model including density-dependent dephasing, advancing understanding of non-linear effects in Rydberg EIT media.

Findings

Model matches experimental data at low probe intensities.

Predicts spectral asymmetry and line broadening at higher intensities.

Deviations at high intensities suggest additional physical effects not yet observed.

Abstract

Light propagation through an ensemble of ultra-cold Rydberg atoms in electromagnetically induced transparency (EIT) configuration is studied. In strongly interacting Rydberg EIT media, non-linear optical effects lead to a non-trivial dependence of the degree of probe beam attenuation on the medium density and on its initial intensity. We develop a Monte Carlo rate equation model that self-consistently includes the effect of the probe beam attenuation to investigate the steady state of the Rydberg medium driven by two laser fields. We compare our results to recent experimental data and to results of other state-of-the-art models for light propagation in Rydberg EIT-media. We find that for low probe field intensities, our results match the experimental data best if a density-dependent dephasing rate is included in the model. At higher probe intensities, our model deviates from other theoretical approaches, as it predicts a spectral asymmetry together with line broadening. These are likely due to off-resonant excitation channels, which however have not been observed in recent experiments. Atomic motion and coupling to additional Rydberg levels are discussed as possible origins for these deviations.