Linewidth of collimated wavelength-converted emission in Rb vapours
Alexander Akulshin, Christopher Perrella, Gar-Wing Truong, Andre, Luiten, Dmitry Budker, Russell McLean

TL;DR
This study measures the spectral linewidth of collimated blue and mid-IR light generated in Rb vapour, showing the linewidth is mainly limited by laser coherence rather than atom-light interaction.
Contribution
It provides the first detailed measurement of the linewidth of collimated mid-IR radiation in Rb vapour, highlighting the influence of laser coherence.
Findings
CBL linewidth is less than 1.3 MHz under various conditions
Linewidth is primarily limited by laser coherence
Upper limit of mid-IR linewidth is several hundred kHz
Abstract
We present a study of the spectral linewidth of collimated blue light (CBL) that results from wave mixing of low-power cw laser radiation at 780 nm and 776 nm and an internally-generated mid-IR field at 5.23 um in Rb vapour. Using a high-finesse Fabry-Perot interferometer the spectral width of the CBL is found to be less than 1.3 MHz for a wide range of experimental conditions. We demonstrate that the CBL linewidth is mainly limited by the temporal coherence of the applied laser fields rather than the atom-light interaction itself. Results obtained with frequency modulated laser light allow an upper limit of several hundred kHz to be set for the linewidth of the collimated mid-IR radiation at 5.23 um, which has not been directly detected.
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