Electronic phase separation due to magnetic polaron formation in the semimetallic ferromagnet EuB$_6$ - A weakly-nonlinear-transport study

TL;DR

This study investigates weakly nonlinear electronic transport in EuB$_6$, revealing how magnetic polaron formation and percolation drive phase transitions and influence resistivity and nonlinear voltage responses.

Contribution

It provides new insights into magnetic polaron dynamics and their role in electronic phase separation in EuB$_6$ through nonlinear transport measurements.

Findings

Onset of nonlinearity coincides with ferromagnetic transition.

Peak in third-harmonic voltage at lower transition.

Linear temperature dependence of nonlinear response peak.

Abstract

We report measurements of weakly nonlinear electronic transport, as measured by third-harmonic voltage generation $V_{3\omega}$, in the low-carrier density semimetallic ferromagnet EuB$_6$, which exhibits an unusual magnetic ordering with two consecutive transitions at $T_{c_1} = 15.6$\,K and $T_{c_2} = 12.5$\,K. Upon cooling in zero magnetic field through the ferromagnetic transition, the dramatic drop in the linear resistivity at the upper transition $T_{c_1}$ coincides with the onset of nonlinearity, and upon further cooling is followed by a pronounced peak in $V_{3 \omega}$ at the lower transition $T_{c_2}$. Likewise, in the paramagnetic regime, a drop of the material's magnetoresistance $R(H)$ precedes a magnetic-field-induced peak in nonlinear transport. A striking observation is a linear temperature dependence of $V_{3\omega}^{\rm peak}(H)$. We suggest a picture where at the upper transition $T_{c_1}$ the coalescing MP form a conducting path giving rise to a strong decrease in the resistance. The MP formation sets in at around $T^\ast \sim 35$\,K below which these entities are isolated and strongly fluctuating, while growing in number. The MP then start to form links at $T_{c_1}$, where percolative electronic transport is observed. The MP merge and start forming a continuum at the threshold $T_{c_2}$. In the paramagnetic temperature regime $T_{c_1} < T < T^\ast$, MP percolation is induced by a magnetic field, and the threshold accompanied by charge carrier delocalization occurs at a single critical magnetization.