Low-temperature heat transport and magnetic-structure transition of the hexagonal TmMnO_3 single crystals

TL;DR

This study investigates low-temperature heat transport and magnetic transitions in TmMnO_3 single crystals, revealing magnetic-field-dependent thermal conductivity and a magnetic-structure transition related to Mn^{3+} spin re-orientation.

Contribution

It provides new insights into the magnetic-field effects on heat transport and magnetic structure transitions in TmMnO_3, highlighting the role of rare-earth ion magnetism.

Findings

Thermal conductivity shows strong magnetic-field dependence.

A dip in ppa(H) at 3.5-4 T for H bla c indicates spin re-orientation.

Magnetothermal conductivity of TmMnO_3 is intermediate among similar compounds.

Abstract

We study the low-temperature heat transport, as well as the magnetization and the specific heat, of TmMnO_3 single crystals to probe the transitions of magnetic structure induced by magnetic field. It is found that the low-T thermal conductivity (\kappa) shows strong magnetic-field dependence and the overall behaviors can be understood in the scenario of magnetic scattering on phonons. In addition, a strong "dip"-like feature shows up in \kappa(H) isotherms at 3.5--4 T for H \parallel c, which is related to a known spin re-orientation of Mn^{3+} moments. The absence of this phenomenon for H \parallel a indicates that the magnetic-structure transition of TmMnO_3 cannot be driven by the in-plane field. In comparison, the magnetothermal conductivity of TmMnO_3 is much larger than that of YMnO_3 but smaller than that of HoMnO_3, indicating that the magnetisms of rare-earth ions are playing the key role in the spin-phonon coupling of the hexagonal manganites.