Indirect RKKY interaction in armchair graphene nanoribbons

TL;DR

This paper investigates the indirect RKKY-like magnetic coupling in armchair graphene nanoribbons, revealing size-dependent oscillations and different distance decay behaviors in semiconducting and metallic cases.

Contribution

It provides a theoretical analysis of RKKY interactions in finite armchair graphene nanoribbons, highlighting quantum size effects and the role of zero-energy states.

Findings

Coupling exhibits Friedel-oscillation-like dependence on impurity position.

Semiconducting nanoribbons show exponential-like distance dependence.

Metallic nanoribbons with zero-energy states have slower decay of coupling.

Abstract

A form of an indirect Ruderman-Kittel-Kasuya-Yosida (RKKY)-like coupling between magnetic on-site impurities in armchair graphene nanoribbons is studied theoretically. The calculations are based on a tight-binding model for a finite nanoribbon system with periodic boundary conditions. A pronounced Friedel-oscillation-like dependence of the coupling magnitude on the impurity position within the nanoribbon resulting from quantum size effects is found and investigated. In particular, the distance dependence of coupling is analysed. For semiconducting nanoribbons, this dependence is exponential-like, resembling the Bloembergen-Rowland interaction. In particular, for metallic nanoribbons, interesting behaviour is found for finite length systems, in which zero-energy states make an important contribution to the interaction. In such situation, the coupling decay with the distance can be then substantially slower.