Light narrowing of magnetic resonances in ensembles of nitrogen-vacancy centers in diamond

TL;DR

This study demonstrates that increasing light power can significantly narrow magnetic resonance linewidths in nitrogen-vacancy centers in diamond, enhancing magnetic sensing sensitivity.

Contribution

It reveals the light-narrowing effect in NV centers and identifies spin-spin interactions as a key factor influencing resonance linewidths.

Findings

Linewidth decreases with increasing light power, achieving over twofold narrowing.

Spin-spin interactions affect lineshape and linewidth.

Light narrowing can optimize magnetic field measurement sensitivity.

Abstract

We investigate optically detected magnetic resonance signals from an ensemble of nitrogen-vacancy centers in diamond. The signals are measured for different light powers and microwave powers, and the contrast and linewidth of the magnetic-resonance signals are extracted. For a wide range of experimental settings of the microwave and light powers, the linewidth decreases with increasing light power, and more than a factor of two "light narrowing" is observed.Furthermore, we identify that spin-spin interaction between nitrogen-vacancy centers and substitutional nitrogen atoms in the diamond leads to changes in the lineshape and the linewidth of the optically detected magnetic-resonance signals. Finally, the importance of the light-narrowing effect for optimizing the sensitivity of magnetic field measurements is discussed.