Implementation of Quantum Logic Gates Using Polar Molecules in Pendular States
Jing Zhu, Sabre Kais, Qi Wei, Dudley Herschbach, Bretislav, Friedrich

TL;DR
This paper proposes a method to implement quantum logic gates using polar molecules in pendular states, employing optimal control theory to achieve high-fidelity operations suitable for quantum computing.
Contribution
It introduces a systematic approach combining pendular states and optimal control theory for implementing quantum gates on polar molecules.
Findings
High-fidelity realization of NOT, Hadamard, and CNOT gates.
Detailed calculations for SrO molecules as qubits.
Use of laser fields optimized via MTOCT for gate operations.
Abstract
We present a systematic approach to implementation of basic quantum logic gates operating on polar molecules in pendular states as qubits for a quantum computer. A static electric field prevents quenching of the dipole moments by rotation, thereby creating the pendular states; also, the field gradient enables distinguishing among qubit sites. Multi-Target Optimal Control Theory (MTOCT) is used as a means of optimizing the initial-to-target transition probability via a laser field. We give detailed calculations for the SrO molecule, a favorite candidate for proposed quantum computers. Our simulation results indicate that NOT, Hadamard and CNOT gates can be realized with high fidelity for such pendular qubit states.
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