Probing the Dynamical Behaviour of Surface Dipoles Through Energy Absorption Interferometry

TL;DR

This paper introduces a method using energy absorption interferometry and simulations with the Discrete Dipole Approximation to analyze the dynamical modes and collective excitations of surface dipoles, revealing long-range coherence effects.

Contribution

The paper demonstrates how to recover dynamical modes of surface dipoles considering interactions using DDA-based simulations and interferometry.

Findings

Revealed long-range coherent phenomena in surface dipoles.

Enabled modeling of diverse objects from photonic films to biomolecules.

Provided a way to analyze collective excitations through energy absorption measurements.

Abstract

Spatial interferometry, based on the measurement of total absorbed power, can be used to determine the state of coherence of the electromagnetic field to which any energy-absorbing structure is sensitive. The measured coherence tensor can be diagonalized to give the amplitude, phase, polarization patterns, and responsivities of the individual electromagnetic modes through which the structure can absorb energy. Because the electromagnetic modes are intimately related to dynamical modes of the system, information about collective excitations can be found. We present simulations, based on the Discrete Dipole Approximation (DDA), showing how the dynamical modes of systems of surface dipoles can be recovered. Interactions are taken into consideration, leading to long-range coherent phenomena, which are revealed by the method. The use of DDA enables the interferometric response of a wide variety of objects to be modeled, from patterned photonic films to biological macromolecules.