Phase Transition in a Out-of-equilibrium Monolayer of Dipolar Vibrated Grains

TL;DR

This study experimentally investigates the phase transition between liquid-like and solid-like states in a vibrated monolayer of magnetized grains, revealing hysteresis, metastability, and nucleation dynamics influenced by magnetic interactions and driving conditions.

Contribution

It provides new insights into the hysteresis and metastability of phase transitions in vibrated magnetic granular monolayers, with a proposed theoretical model for cluster growth.

Findings

Hysteresis observed in solid-liquid transition with critical acceleration values.

Metastable cluster nucleation after rapid quench from high acceleration.

Cluster growth follows a stretched exponential law, with a theoretical model proposed.

Abstract

We report an experimental study on the transition between a disordered liquid-like state and a ordered solid-like one, in a collection of magnetically interacting macroscopic grains. A monolayer of magnetized particles is vibrated vertically at a moderate density. At high excitation a disordered, liquid-like state is observed. When the driving dimensionless acceleration $\Gamma$ is quasi-statically reduced, clusters of ordered grains grow below a critical value $\Gamma_{\rm c}$. These clusters have a well defined hexagonal and compact structure. If the driving is subsequently increased, these clusters remain stable up to a higher critical value $\Gamma_{\rm l}$. Thus, the solid-liquid transition exhibits an hysteresis cycle. However, the lower onset $\Gamma_c$ is not well defined as it depends strongly on the acceleration ramp speed and also on the magnetic interaction strength. Metastability is observed when the driving is rapidly quenched from high acceleration, $\Gamma > \Gamma_{\rm l}$, to a low final excitation $\Gamma_q$. After this quench, solid clusters nucleate after a time lag $\tau_o$, either immediately ($\tau_o = 0$) or after some time lag ($\tau_o>0$) that can vary from seconds up to several hundreds of seconds. The immediate growth occurs below a particular acceleration value $\Gamma_s$ ($\lesssim \Gamma_c$). In all cases, for $t \geq \tau_o$ solid cluster's temporal growth can be phenomenologically described by a stretched exponential law. Finally, by taking into account the finite size of our system and by using simple assumptions we propose an alternative tractable theoretical model that reproduces cluster's growth, but which analytical form is not a stretched exponential law.