Dynamic phase transition properties and hysteretic behavior of a ferrimagnetic core-shell nanoparticle in the presence of a time dependent magnetic field

TL;DR

This study investigates the dynamic phase transitions, hysteresis, and magnetic properties of a ferrimagnetic core-shell nanoparticle under high-frequency oscillating magnetic fields using Monte Carlo simulations.

Contribution

It provides new insights into the phase diagrams, hysteresis behavior, and size effects of ferrimagnetic nanoparticles subjected to ultrafast switching fields.

Findings

Existence of triple hysteresis loops due to core and interface interactions.

Dynamic phase transition from paramagnetic to ordered phase with increasing shell thickness.

Magnetic properties depend strongly on particle size and field frequency.

Abstract

We have presented dynamic phase transition features and stationary-state behavior of a ferrimagnetic small nanoparticle system with a core-shell structure. By means of detailed Monte Carlo simulations, a complete picture of the phase diagrams and magnetization profiles have been presented and the conditions for the occurrence of a compensation point $T_{comp}$ in the system have been investigated. According to N\'{e}el nomenclature, the magnetization curves of the particle have been found to obey P-type, N-type and Q-type classification schemes under certain conditions. Much effort has been devoted to investigation of hysteretic response of the particle and we observed the existence of triple hysteresis loop behavior which originates from the existence of a weak ferromagnetic core coupling $J_{c}/J_{sh}$, as well as a strong antiferromagnetic interface exchange interaction $J_{int}/J_{sh}$. Most of the calculations have been performed for a particle in the presence of oscillating fields of very high frequencies and high amplitudes in comparison with exchange interactions which resembles a magnetic system under the influence of ultrafast switching fields. Particular attention has also been paid on the influence of the particle size on the thermal and magnetic properties, as well as magnetic features such as coercivity, remanence and compensation temperature of the particle. We have found that in the presence of ultrafast switching fields, the particle may exhibit a dynamic phase transition from paramagnetic to a dynamically ordered phase with increasing ferromagnetic shell thickness.