Electron doping evolution of the anisotropic spin excitations in BaFe2-xNixAs2

TL;DR

This study uses inelastic neutron scattering to explore how Ni-doping affects low-energy spin excitations in BaFe2-xNixAs2 across different doping levels, revealing changes in magnetic exchange and spin resonance linked to superconductivity.

Contribution

It provides a systematic experimental investigation of Ni-doping effects on spin excitations, supporting an itinerant electron model and RPA calculations for this material.

Findings

Spin excitation widths increase linearly with doping, faster transversely.

A neutron spin resonance appears near optimal doping and vanishes with decreasing Tc.

Overdoped samples show incommensurate spin excitations consistent with RPA predictions.

Abstract

We use inelastic neutron scattering to systematically investigate the Ni-doping evolution of the low-energy spin excitations in BaFe2-xNixAs2 spanning from underdoped antiferromagnet to overdoped superconductor (0.03< x < 0.18). In the undoped state, the low-energy (<80 meV) spin waves of BaFe2As2 form transversely elongated ellipses in the [H, K] plane of the reciprocal space. Upon Ni-doping, the c-axis magnetic exchange coupling is rapidly suppressed and the momentum distribution of spin excitations in the [H, K] plane is enlarged in both the transverse and longitudinal directions with respect to the in-plane AF ordering wave vector of the parent compound. As a function of increasing Ni-doping x, the spin excitation widths increase linearly but with a larger rate along the transverse direction. These results are in general agreement with calculations of dynamic susceptibility based on the random phase approximation (RPA) in an itinerant electron picture. For samples near optimal superconductivity at x= 0.1, a neutron spin resonance appears in the superconducting state. Upon further increasing the electron-doping to decrease the superconducting transition temperature Tc, the intensity of the low-energy magnetic scattering decreases and vanishes concurrently with vanishing superconductivity in the overdoped side of the superconducting dome. Comparing with the low-energy spin excitations centered at commensurate AF positions for underdoped and optimally doped materials (x<0.1), spin excitations in the over-doped side (x=0.15) form transversely incommensurate spin excitations, consistent with the RPA calculation. Therefore, the itinerant electron approach provides a reasonable description to the low-energy AF spin excitations in BaFe2-xNixAs2.