Nuclear spin physics in quantum dots: an optical investigation

TL;DR

This paper reviews how optical techniques are used to manipulate and measure nuclear spins in quantum dots, highlighting recent advances in controlling nuclear spin polarization and fluctuations to improve electron spin coherence for quantum information applications.

Contribution

It provides a comprehensive overview of experimental methods for optical addressing of nuclear spins in quantum dots and discusses their implications for quantum coherence and future research directions.

Findings

Optical methods can establish non-zero nuclear spin polarization.

Techniques have been developed to reduce nuclear spin fluctuations.

These advances improve electron spin coherence in quantum dots.

Abstract

The mesoscopic spin system formed by the 10E4-10E6 nuclear spins in a semiconductor quantum dot offers a unique setting for the study of many-body spin physics in the condensed matter. The dynamics of this system and its coupling to electron spins is fundamentally different from its bulk counter-part as well as that of atoms due to increased fluctuations that result from reduced dimensions. In recent years, the interest in studying quantum dot nuclear spin systems and their coupling to confined electron spins has been fueled by its direct implication for possible applications of such systems in quantum information processing as well as by the fascinating nonlinear (quantum-)dynamics of the coupled electron-nuclear spin system. In this article, we review experimental work performed over the last decades in studying this mesoscopic,coupled electron-nuclear spin system and discuss how optical addressing of electron spins can be exploited to manipulate and read-out quantum dot nuclei. We discuss how such techniques have been applied in quantum dots to efficiently establish a non-zero mean nuclear spin polarization and, most recently, were used to reduce fluctuations of the average quantum dot nuclear spin orientation. Both results in turn have important implications for the preservation of electron spin coherence in quantum dots, which we discuss. We conclude by speculating how this recently gained understanding of the quantum dot nuclear spin system could in the future enable experimental observation of quantum-mechanical signatures or possible collective behavior of mesoscopic nuclear spin ensembles.