Potential antiferromagnetic fluctuations in hole-doped iron-pnictide superconductor Ba_{1-x}K_{x}Fe_{2}As_{2} studied by ^{75}As nuclear magnetic

TL;DR

This study uses ^{75}As NMR and NQR to investigate antiferromagnetic fluctuations and superconducting gap structures in Ba_{1-x}K_{x}Fe_{2}As_{2}, revealing doping-dependent magnetic and electronic behaviors.

Contribution

It provides detailed insights into the evolution of magnetic fluctuations and superconducting gaps across different doping levels in Ba_{1-x}K_{x}Fe_{2}As_{2} using NMR and NQR techniques.

Findings

Large antiferromagnetic fluctuations observed for all x.

Superconducting gaps decrease with increasing x, nearly vanishing for x > 0.6.

Stripe-type AF fluctuations dominate in the system.

Abstract

We have performed ^{75}As nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) on single crystalline Ba_{1-x}K_{x}Fe_{2}As_{2} for x = 0.27-1. ^{75}As nuclear quadruple resonance frequency ({\nu}_{Q}) increases linearly with increasing x. The Knight shift K in normal state shows Pauli paramagnetic behavior with slight temperature T dependence. The value of K increases gradually with increasing x. By contrast, nuclear spin- lattice relaxation rate 1/T_{1} in normal state has a large T-dependence, which indicates existence of large antiferomagnetic (AF) spin fluctuations for all x. The T-dependence of 1/T_{1} shows a gap-like behavior below approximately 100 K for 0.6 < x < 0.9. These behaviors are well explained by the change of band structure with expansion of hole Fermi surfaces and shrink and disappearance of electron Fermi surfaces at Brillouin zone (BZ) with increasing x. The anisotropy of 1/T_{1}, represented by a ratio of 1/T_{1ab} to 1/T_{1c}, is always larger than 1 for all x, which indicates that the stripe-type AF fluctuations is dominant in this system. The K in superconducting (SC) state decreases, which corresponds to appearance of spin-singlet superconductivity. The T dependence of 1/T_{1} in SC state indicates multiple-SC-gap feature. A simple two gap model analysis shows that the larger superconducting gap gradually decreases with increasing x from 0.27 to 1 and smaller gap decreases rapidly and nearly vanishes for x > 0.6 where the electron pockets in BZ disappear.