Local Quantum Criticality of an Iron-Pnictide Tetrahedron

TL;DR

This paper investigates the quantum critical behavior of an isolated iron-arsenide tetrahedron within a metallic environment, revealing non-Fermi liquid states that could influence superconductivity in iron-based materials.

Contribution

It introduces a theoretical study of spin and orbital interactions in an iron-arsenide tetrahedron, highlighting the role of orbital quenching and non-Fermi liquid states in superconductivity.

Findings

Orbital degrees of freedom quench at high temperatures.

Suppressed spin Kondo effect due to Hund's coupling.

Potential link between critical states and superconductivity.

Abstract

Motivated by the close correlation between transition temperature ($T_c$) and the tetrahedral bond angle of the As-Fe-As layer observed in the iron-based superconductors, we study the interplay between spin and orbital physics of an isolated iron-arsenide tetrahedron embedded in a metallic environment. Whereas the spin Kondo effect is suppressed to low temperatures by Hund's coupling, the orbital degrees of freedom are expected to quantum mechanically quench at high temperatures, giving rise to an overscreened, non-Fermi liquid ground-state. Translated into a dense environment, this critical state may play an important role in the superconductivity of these materials.