Magnons and electromagnons in a spin-lattice-coupled frustrated magnet CuFeO2 as seen via inelastic neutron scattering

TL;DR

This study investigates the detailed spin-wave excitations and electromagnon modes in CuFeO2, revealing how spin-lattice interactions influence magnon behavior and electric-field-active excitations in a frustrated magnet.

Contribution

The paper develops a detailed model Hamiltonian that accurately reproduces neutron scattering data and elucidates the nature of magnon and electromagnon modes in CuFeO2.

Findings

Resolved fine structures of spin-wave branches near the zone center.

Successfully modeled spin-wave dispersion and intensity maps.

Identified the roles of collinear and noncollinear spin modes in electromagnon activity.

Abstract

We have investigated spin-wave excitations in a four-sublattice (4SL) magnetic ground state of a frustrated magnet CuFeO2, in which `electromagnon' (electric-field-active magnon) excitation has been discovered by recent terahertz time-domain spectroscopy [Seki et al. Phys. Rev. Lett. 105 097207 (2010)]. In previous study, we have identified two spin-wave branches in the 4SL phase by means of inelastic neutron scattering measurements under applied uniaxial pressure. [T. Nakajima et al. J. Phys. Soc. Jpn. 80 014714 (2011) ] In the present study, we have performed high-energy-resolution inelastic neutron scattering measurements in the 4SL phase, resolving fine structures of the lower-energy spin-wave branch near the zone center. Taking account of the spin-driven lattice distortions in the 4SL phase, we have developed a model Hamiltonian to describe the spin-wave excitations. The determined Hamiltonian parameters have successfully reproduced the spin-wave dispersion relations and intensity maps obtained in the inelastic neutron scattering measurements. The results of the spin-wave analysis have also revealed physical pictures of the magnon and electromagnon modes in the 4SL phase, suggesting that collinear and noncollinear characters of the two spin-wave modes are the keys to understand the dynamical coupling between the spins and electric dipole moments in this system.