Invariant barriers to reactive front propagation in fluid flows

TL;DR

This paper develops a theory and conducts experiments on reaction front dynamics in vortex flows, identifying invariant barriers called BIMs that control front propagation.

Contribution

It introduces burning invariant manifolds (BIMs) as a new concept to describe barriers to reactive front propagation in fluid flows, supported by theoretical and experimental evidence.

Findings

BIMs act as one-sided barriers to front propagation.

BIMs are fixed or oscillate periodically depending on flow type.

Experimental measurements confirm BIMs' role as propagation barriers.

Abstract

We present theory and experiments on the dynamics of reaction fronts in two-dimensional, vortex-dominated flows, for both time-independent and periodically driven cases. We find that the front propagation process is controlled by one-sided barriers that are either fixed in the laboratory frame (time-independent flows) or oscillate periodically (periodically driven flows). We call these barriers \emph{burning invariant manifolds} (BIMs), since their role in front propagation is analogous to that of invariant manifolds in the transport and mixing of passive impurities under advection. Theoretically, the BIMs emerge from a dynamical systems approach when the advection-reaction-diffusion dynamics is recast as an ODE for front element dynamics. Experimentally, we measure the location of BIMs for several laboratory flows and confirm their role as barriers to front propagation.