Huge Positive Magnetoresistance in Antiferromagnetic Double Perovskite Metals

TL;DR

This paper reveals that antiferromagnetic double perovskite metals exhibit extremely large positive magnetoresistance due to field-induced suppression of antiferromagnetic order, with potential applications in magnetic sensing.

Contribution

It introduces a novel mechanism for positive magnetoresistance in antiferromagnetic metals, demonstrated through a spin-fermion model, and suggests broader applicability beyond double perovskites.

Findings

Resistance ratio exceeds tenfold at moderate fields.

Almost twofold resistance increase persists with 25% antisite disorder.

Mechanism is general and applicable to other local moment metals.

Abstract

Metals with large positive magnetoresistance are rare. We demonstrate that antiferromagnetic metallic states, as have been predicted for the double perovskites, are excellent candidates for huge positive magnetoresistance. An applied field suppresses long range antiferromagnetic order leading to a state with short range antiferromagnetic correlations that generate strong electronic scattering. The field induced resistance ratio can be more than tenfold, at moderate field, in a structurally ordered system, and continues to be almost twofold even in systems with upto 25 % antisite disorder. Although our explicit demonstration is in the context of a two dimensional spin-fermion model of the double perovskites, the mechanism we uncover is far more general, complementary to the colossal negative magnetoresistance process, and would operate in other local moment metals that show a field driven suppression of non-ferromagnetic order.