Harmonic generation and energy transport in dielectric and semiconductors at visible and UV wavelengths: the case of GaP

TL;DR

This paper investigates how harmonic pulses propagate in dielectrics and semiconductors like GaP at visible and UV wavelengths, revealing phase locking effects that enable energy transport despite absorption.

Contribution

It demonstrates that phase locking allows harmonic signals to bypass absorption in GaP, opening new avenues in ultrafast nonlinear optics and nano-plasmonics.

Findings

Harmonic signals can propagate without absorption via phase locking.

Energy and momentum transport exhibit unusual, anomalous behavior.

Potential for new applications in ultrafast optics and nano-plasmonics.

Abstract

We study inhibition of absorption, transparency, energy and momentum transport of the inhomogeneous component of harmonic pulses in dielectrics and semiconductors, at visible and UV wavelengths, focusing on materials like GaP. In these spectral regions GaP is characterized by large absorption, metallic behavior or a combination of both. We show that phase locking causes the generated inhomogeneous signals to propagate through a bulk metallic medium without being absorbed, that is occurs even in centrosymmetric materials via the magnetic Lorentz force, and that the transport of energy and momentum is quite peculiar and seemingly anomalous. These results make it clear that there are new opportunities in ultrafast nonlinear optics and nano-plasmonics in new wavelength ranges.