Topological and magnetic phases of interacting electrons in the pyrochlore iridates

TL;DR

This paper models interacting electrons in pyrochlore iridates with strong spin-orbit coupling, predicting novel quantum phase transitions, magnetic orders, and the potential realization of Weyl semi-metal phases driven by electron correlations.

Contribution

It introduces a model emphasizing direct hopping effects and explores the emergence of topological and magnetic phases, including Weyl semi-metal states, across different interaction strengths.

Findings

Identification of topological insulator and metallic phases at weak coupling.

Prediction of magnetic orders, including all-in/all-out pattern.

Realization of Weyl semi-metal phase in correlated magnetic insulators.

Abstract

We construct a model for interacting electrons with strong spin orbit coupling in the pyrochlore iridates. We establish the importance of the direct hopping process between the Ir atoms and use the relative strength of the direct and indirect hopping as a generic tuning parameter to study the correlation effects across the iridates family. We predict novel quantum phase transitions between conventional and/or topologically non-trivial phases. At weak coupling, we find topological insulator and metallic phases. As one increases the interaction strength, various magnetic orders emerge. The topological Weyl semi-metal phase is found to be realized in these different orders, one of them being the all-in/all-out pattern. Our findings establish the possible magnetic ground states for the iridates and suggest the generic presence of the Weyl semi-metal phase in correlated magnetic insulators on the pyrochlore lattice. We discus the implications for existing and future experiments.