An Athermal Brittle to Ductile Transition in Amorphous Solids

TL;DR

This paper introduces an athermal transition from brittle to ductile behavior in amorphous solids, explained through the increase in plastic modes as a function of inter-particle potential cutoff length, supported by numerical simulations.

Contribution

It presents the first analysis of an athermal brittle to ductile transition based on potential cutoff length, expanding understanding beyond temperature-dependent mechanisms.

Findings

Ductility increases with larger potential cutoff length.

Plastic mode density correlates with ductile behavior.

Resolves the experimental-molecular dynamics fracture paradox.

Abstract

Brittle materials exhibit sharp dynamical fractures when meeting Griffith's criterion, whereas ductile materials blunt a sharp crack by plastic responses. Upon continuous pulling ductile materials exhibit a necking instability which is dominated by a plastic flow. Usually one discusses the brittle to ductile transition as a function of increasing temperature. We introduce an athermal brittle to ductile transition as a function of the cut-off length of the inter-particle potential. On the basis of extensive numerical simulations of the response to pulling the material boundaries at a constant speed we offer an explanation of the onset of ductility via the increase in the density of plastic modes as a function of the potential cutoff length. Finally we can resolve an old riddle: in experiments brittle materials can be strained under grip boundary conditions, and exhibit a dynamic crack when cut with a sufficiently long initial slot. Mysteriously, in molecular dynamics simulations it appeared that cracks refused to propagate dynamically under grip boundary conditions, and continuous pulling was necessary to achieve fracture. We argue that this mystery is removed when one understands the distinction between brittle and ductile athermal amorphous materials.