Power law decay and phase rigidity for large-amplitude coherent phonons in bismuth at helium temperature: Possible evidence for transient supersolid state

TL;DR

This paper investigates how intense ultrafast laser excitation induces unusual lattice dynamics in bismuth, revealing potential signs of a transient supersolid state through anomalous phonon decay and phase rigidity.

Contribution

It presents experimental evidence of large-amplitude coherent phonons exhibiting decay and phase rigidity, suggesting the possible realization of a transient supersolid state in bismuth.

Findings

Observation of anomalous decay of coherent phonons

Detection of phase rigidity at high excitation levels

Evidence supporting transient supersolid behavior

Abstract

Intense ultrafast laser excitation can produce transient states of condensed matter that would otherwise be inaccessible. At high excitation level, the interatomic forces can be altered resulting in an unusual lattice dynamics. Here we report the study of coherent lattice dynamics in Bi made for various excitation levels at helium temperature. We demonstrate that under certain conditions the fully symmetric phonons of large amplitude exhibit anomalous decay and phase rigidity, both of which possibly signaling the attainment of transient supersolid state.