Excited State Quantum Couplings and Optical Switching of an Artificial Molecule

TL;DR

This study investigates the optical properties and excited state couplings of a tunable quantum dot molecule, demonstrating hybridized states and a high-contrast optical switching mechanism.

Contribution

It reveals the formation of hybridized electron states and demonstrates a novel electrically tunable optical switching method in a quantum dot molecule.

Findings

Hybridized electron states cause anticrossings in excited state transitions.

Electrical tuning adjusts the energy separation of exciton states.

Achieved 88% contrast in laser-induced optical switching.

Abstract

We optically probe the spectrum of ground and excited state transitions of an individual, electrically tunable self-assembled quantum dot molecule. Photocurrent absorption measurements show that the spatially direct neutral exciton transitions in the upper and lower dots are energetically separated by only ~2 meV. Excited state transitions ~8-16 meV to higher energy exhibit pronounced anticrossings as the electric field is tuned due to the formation of hybridized electron states. We show that the observed excited state transitions occur between these hybridized electronic states and different hole states in the upper dot. By simultaneously pumping two different excited states with two laser fields we demonstrate a strong (88% on-off contrast) laser induced switching of the optical response. The results represent an electrically tunable, discrete coupled quantum system with a conditional optical response.