X-ray Near Field Speckle: Implementation and Critical Analysis

TL;DR

This paper reports the implementation of x-ray near-field speckle (XNFS) at a synchrotron source, demonstrating its ability to study static and dynamic structures at larger length scales than traditional methods, with a critical analysis of its limitations.

Contribution

The paper introduces a new implementation of XNFS at a synchrotron, including a high-resolution detector setup, and provides a detailed analysis of its capabilities and limitations.

Findings

Successfully implemented XNFS at 8-ID-I beamline.

Demonstrated study of colloidal structures and dynamics.

Identified limitations of the XNFS technique.

Abstract

We have implemented the newly-introduced, coherence-based technique of x-ray near-field speckle (XNFS) at 8-ID-I at the Advanced Photon Source. In the near field regime of high-brilliance synchrotron x-rays scattered from a sample of interest, it turns out, that, when the scattered radiation and the main beam both impinge upon an x-ray area detector, the measured intensity shows low-contrast speckles, resulting from interference between the incident and scattered beams. We built a micrometer-resolution XNFS detector with a high numerical aperture microscope objective and demonstrate its capability for studying static structures and dynamics at longer length scales than traditional far field x-ray scattering techniques. Specifically, we characterized the structure and dynamics of dilute silica and polystyrene colloidal samples. Our study reveals certain limitations of the XNFS technique, which we discuss.