A pulsating regime of magnetic deflagration

TL;DR

This paper investigates the stability of magnetic deflagration fronts in molecular magnets, revealing a pulsating regime triggered when the energy barrier exceeds a critical ratio to Zeeman energy, with analytical and numerical analysis of the instability.

Contribution

It introduces the concept of a pulsating regime in magnetic deflagration and provides analytical and numerical analysis of the instability mechanism.

Findings

Stationary deflagration becomes unstable above a critical Zeldovich number.

A pulsating regime of magnetic deflagration is identified and characterized.

Parameter conditions for observing pulsating regimes are discussed.

Abstract

The stability of a magnetic deflagration front in a collection of molecular magnets, such as Mn_12-acetate, is considered. It is demonstrated that stationary deflagration is unstable with respect to one-dimensional perturbations if the energy barrier of the magnets is sufficiently high in comparison with the release of Zeeman energy at the front; their ratio may be interpreted as an analogue to the Zeldovich number, as found in problems of combustion. When the Zeldovich number exceeds a certain critical value, a stationary deflagration front becomes unstable and propagates in a pulsating regime. Analytical estimates for the critical Zeldovich number are obtained. The linear stage of the instability is investigated numerically by solving the eigenvalue problem. The nonlinear stage is studied using direct numerical simulations. The parameter domain required for experimental observations of the pulsating regime is discussed.