Atomic interferometer measurements of Berry's and Aharonov-Anandan's phases for isolated spins S > 1/2 non-linearly coupled to external fields

TL;DR

This paper proposes experimental methods to observe Berry's and Aharonov-Anandan's phases in high-spin systems with complex couplings, using alkali atoms and numerical simulations to address practical challenges.

Contribution

It introduces feasible experimental schemes for measuring geometric phases in spins greater than 1, including non-adiabatic corrections and alternative atomic candidates.

Findings

Non-adiabatic corrections can be kept below 0.1%

Proposed use of $^{87}$Rb and chromium atoms as candidates

Extension of phase measurement techniques beyond spin-1/2

Abstract

The aim of the present paper is to propose experiments for observing the significant features of Berry's phases for S>1, generated by spin-Hamiltonians endowed with two couplings, a magnetic dipole and an electric quadrupole one with external B and E fields, as theoretically studied in our previous work. The fields are assumed orthogonal, this mild restriction leading to geometric and algebraic simplifications. Alkali atoms appear as good candidates for interferometric measurements but there are challenges to be overcome. The only practical way to generate a suitable E-field is to use the ac Stark effect which induces an instability of the dressed atom. Besides atom loss, this might invalidate Berry's phase derivation but this latter problem can be solved by an appropriate detuning. The former puts an upper limit to the cycle duration, which is bounded below by the adiabatic condition. By relying upon our previous analysis of the non-adiabatic corrections, we have been able to reach a compromise for the $^{87}$Rb hf level F=2, m=0 state, which is our candidate for an interferometric measurement of the exotic Berry's phase generated by a rotation of the E-field around the fixed B-field. By a numerical simulation we have shown that the non-adiabatic corrections can be kept below the 0.1% level. As an alternative candidate, we discuss the chromium ground state J=S=3, where the instability problem is easily solved. We make a proposal to extend the measurement of Aharonov-Anandan's phase beyond S=1/2 to the $^{87}$Rb hf level F=m=1, by constructing, with the help of light-shifts, a Hamiltonian able to perform a parallel transport along a closed circuit upon the density matrix space, without any adiabatic constraint. In Appendix A, Berry's phase difference for S=3/2 and 1/2, m=1/2 states is used to perform an entanglement of 3 Qbits.