Transport Spin Polarization of High-Curie Temperature MnBi Films

TL;DR

This study investigates the high-temperature ferromagnetic MnBi films, measuring their structural, magnetic, and transport properties, including a significant transport spin polarization, supported by experimental data and relativistic band structure calculations.

Contribution

It provides the first detailed measurement of transport spin polarization in MnBi films and correlates it with their magnetic properties, supported by theoretical calculations.

Findings

Transport spin polarization of 51-63% observed.

High Curie temperature of 628K confirmed.

Band structure calculations explain high spin polarization.

Abstract

We report on the study of the structural, magnetic and transport properties of highly textured MnBi films with the Curie temperature of 628K. In addition to detailed measurements of resistivity and magnetization, we measure transport spin polarization of MnBi by Andreev reflection spectroscopy and perform fully relativistic band structure calculations of MnBi. A spin polarization from 51\pm1 to 63\pm1% is observed, consistent with the calculations and with an observation of a large magnetoresistance in MnBi contacts. The band structure calculations indicate that, in spite of almost identical densities of states at the Fermi energy, the large disparity in the Fermi velocities leads to high transport spin polarization of MnBi. The correlation between the values of magnetization and spin polarization is discussed.