Effect of Interlayer Shear to Graphene Resonators

TL;DR

This paper investigates how interlayer shear affects the resonant frequencies of multilayer graphene nanostrips, revealing deviations from classical theory and proposing a new multi-beam shear model validated by molecular dynamics simulations.

Contribution

It introduces a multi-beam shear model that accurately predicts the vibrational behavior of multilayer graphene nano-strips considering interlayer shear effects.

Findings

Resonant frequency scales as l^-1.36, differing from classical theory.

Interlayer shear modulus is much smaller than intralayer Young's modulus.

The proposed model matches MD simulation results without fitting parameters.

Abstract

Graphene nanostrips with single or a few layers can be made into bending resonators with extremely high sensitivity to environment changes. In this work we study the effect of interlayer shear on resonant frequencies f of graphene nanostrips, via both molecular dynamics (MD) simulation and elastic model analysis incorporating interlayer shear. Contrary to the classical thin beam theory prediction f~nl^-2 (l is beam length and n layer number), MD simulation results reveal very different dependences, f~l^-1.36 and f - fmono~(n-1)/n (fmono is frequency of the monolayer beam). Interlayer shear modulus of multilayer graphene strips is much smaller than their intralayer Young's modulus, and the weak interlayer interaction can not maintain the registry between the carbon atoms in adjacent layers. Large shear deformation occurs during vibration of multilayer graphene nano-strips. Therefore we propose a multi-beam shear model (MBSM) with the interlayer shear energy of multilayer graphene nano-strips taken into account. It makes predictions consistent excellently with direct MD simulations without any fitting parameter required. The results are of importance for various applications of multi-layer graphene nano-strips, such as in nano-electromechanical devices including resonators, sensors and actuators, where interlayer shear has apparent impacts to deformation, vibration, and energy dissipation processes.