Electron transport and anisotropy of the upper critical magnetic field in a Ba0.68K0.32Fe2As2 single crystals

TL;DR

This study investigates the electron transport and magnetic field anisotropy in Ba0.68K0.32Fe2As2 single crystals, revealing anisotropic upper critical fields and detailed phase diagrams, challenging previous assumptions of isotropy in similar compounds.

Contribution

It provides the first detailed measurements of Hc2(T) anisotropy in optimally doped Ba0.68K0.32Fe2As2, showing anisotropy persists down to low temperatures, unlike underdoped counterparts.

Findings

Hc2(T) is anisotropic in optimally doped samples.

Anisotropy parameter γ is about 2.2 at Tc.

Hc2 lines show concave curvature and saturation at low temperatures.

Abstract

Early work on the iron-arsenide compounds supported the view, that a reduced dimensionality might be a necessary prerequisite for high-Tc superconductivity. Later, however, it was found that the zero-temperature upper critical magnetic field, Hc2(0), for the 122 iron pnictides is in fact rather isotropic. Here, we report measurements of the temperature dependence of the electrical resistivity, \Gamma(T), in Ba0.5K0.5Fe2As2 and Ba0.68K0.32Fe2As2 single crystals in zero magnetic field and for Ba0.68K0.32Fe2As2 as well in static and pulsed magnetic fields up to 60 T. We find that the resistivity of both compounds in zero field is well described by an exponential term due to inter-sheet umklapp electron-phonon scattering between light electrons around the M point to heavy hole sheets at the \Gamma point in reciprocal space. From our data, we construct an H-T phase diagram for the inter-plane (H || c) and in-plane (H || ab) directions for Ba0.68K0.32Fe2As2. Contrary to published data for underdoped 122 FeAs compounds, we find that Hc2(T) is in fact anisotropic in optimally doped samples down to low temperatures. The anisotropy parameter, {\gamma} = Habc2/Hcc2, is about 2.2 at Tc. For both field orientations we find a concave curvature of the Hc2 lines with decreasing anisotropy and saturation towards lower temperature. Taking into account Pauli spin paramagnetism we perfectly can describe Hc2(T) and its anisotropy.