The Jones-Hore theory of radical-ion-pair reactions is not self-consistent
I. K. Kominis
TL;DR
The paper critiques the Jones-Hore theory of radical-ion-pair reactions, demonstrating that its master equation lacks self-consistency, which questions its validity in describing these reactions.
Contribution
It identifies fundamental inconsistencies in the Jones-Hore master equation, challenging its use in modeling radical-ion-pair reactions.
Findings
The Jones-Hore master equation is not self-consistent.
This inconsistency undermines the theory's validity.
The paper calls for revised theoretical frameworks.
Abstract
It is shown that the master equation introduced by Jones & Hore and purported to describe radical-ion-pair reactions is not self-consistent.
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Taxonomy
TopicsSpectroscopy and Quantum Chemical Studies · Advanced Chemical Physics Studies · Photochemistry and Electron Transfer Studies