Drude Conductivity of Dirac Fermions in Graphene

TL;DR

This paper reports the first measurements of graphene's high-frequency conductivity from THz to mid-IR, revealing Drude-like behavior and unexpected reductions in conductivity strength, highlighting many-body effects and interactions beyond existing theories.

Contribution

It provides novel experimental data on graphene's high-frequency conductivity and uncovers discrepancies with theoretical predictions, emphasizing the importance of many-body effects.

Findings

Conductivity exhibits Drude-like frequency dependence.

Conductivity increases dramatically at THz frequencies.

Absolute conductivity strength is lower than predicted by theory.

Abstract

Electrons moving in graphene behave as massless Dirac fermions, and they exhibit fascinating low-frequency electrical transport phenomena. Their dynamic response, however, is little known at frequencies above one terahertz (THz). Such knowledge is important not only for a deeper understanding of the Dirac electron quantum transport, but also for graphene applications in ultrahigh speed THz electronics and IR optoelectronics. In this paper, we report the first measurement of high-frequency conductivity of graphene from THz to mid-IR at different carrier concentrations. The conductivity exhibits Drude-like frequency dependence and increases dramatically at THz frequencies, but its absolute strength is substantially lower than theoretical predictions. This anomalous reduction of free electron oscillator strength is corroborated by corresponding changes in graphene interband transitions, as required by the sum rule. Our surprising observation indicates that many-body effects and Dirac fermion-impurity interactions beyond current transport theories are important for Dirac fermion electrical response in graphene.