Atomic decay near a quantized medium of absorbing scatterers

TL;DR

This paper investigates how an excited atom's decay rate is affected by a nearby medium of absorbing and scattering spheres, revealing surface effects and the interplay of scattering and absorption using a quantum-electrodynamical model.

Contribution

It introduces a quantum-electrodynamical model to analyze atomic decay near a complex medium with both scattering and absorption, highlighting surface effects and limitations of bulk susceptibility models.

Findings

Surface effects influence atomic decay rates.

Absorption and scattering interplay affects decay properties.

Bulk susceptibility alone does not fully describe decay modifications.

Abstract

The decay of an excited atom in the presence of a medium that both scatters and absorbs radiation is studied with the help of a quantum-electrodynamical model. The medium is represented by a half space filled with a randomly distributed set of non-overlapping spheres, which consist of a linear absorptive dielectric material. The absorption effects are described by means of a quantized damped-polariton theory. It is found that the effective susceptibility of the bulk does not fully account for the medium-induced change in the atomic decay rate. In fact, surface effects contribute to the modification of the decay properties as well. The interplay of scattering and absorption in the total decay rate is discussed.