Orbital Ordering and Unfrustrated $(\pi,0)$ Magnetism from Degenerate Double Exchange in the Iron Pnictides

TL;DR

This paper explains the magnetic excitations in iron pnictides using a degenerate double-exchange model, revealing unfrustrated stripe antiferromagnetism and agreement with neutron scattering data.

Contribution

It introduces a degenerate double-exchange model that accounts for orbital degeneracy and magnetic order in iron pnictides, highlighting the role of ferro-orbital order and anisotropic couplings.

Findings

Magnetic excitation spectra show increased energies at Néel wave vector.

Spectra fit to a spin-only model with strong spatial anisotropy.

Effective couplings along chains are negative, indicating unfrustrated stripe order.

Abstract

The magnetic excitations of the iron pnictides are explained within a degenerate double-exchange model. The local-moment spins are coupled by superexchanges $J_1$ and $J_2$ between nearest and next-nearest neighbors, respectively, and interact with the itinerant electrons of the degenerate $d_{xz}$ and $d_{yz}$ orbitals via a ferromagnetic Hund exchange. The latter stabilizes $(\pi,0)$ stripe antiferromagnetism due to emergent ferro-orbital order and the resulting kinetic energy gain by hopping preferably along the ferromagnetic spin direction. Taking the quantum nature of the spins into account, we calculate the magnetic excitation spectra in the presence of both, super- and double-exchange. A dramatic increase of the spin-wave energies at the competing N\'eel ordering wave vector is found, in agreement with recent neutron scattering data. The spectra are fitted to a spin-only model with a strong spatial anisotropy and additional longer ranged couplings along the ferromagnetic chains. Over a realistic parameter range, the effective couplings along the chains are negative corresponding to unfrustrated stripe antiferromagnetism.