Anisotropic Connectivity and its Influence on Critical Current Densities, Irreversibility Fields, and Flux Creep in In-Situ-Processed MgB2 Strands

TL;DR

This study investigates how anisotropic microstructure in in-situ MgB2 strands affects critical current density, irreversibility fields, and flux creep, revealing microstructural influences on superconducting properties and measurement discrepancies.

Contribution

It uncovers the fibrous microstructure's role in causing differences between transport and magnetic measurements of critical currents and irreversibility fields in MgB2 strands.

Findings

Transport and magnetic measurements show significant differences at higher fields.

Fibrous microstructure causes anisotropic connectivity affecting superconducting properties.

Microstructure influences estimated pinning potentials and flux creep behavior.

Abstract

The anisotropy of the critical current density (Jc) and its influence on measurement of irreversibility field (Birr) has been investigated for high quality, in-situ MgB2 strands. Comparison of transport and magnetization measurements has revealed the onset of a regime where large differences exist between transport and magnetically measured values of the critical current density and Birr. These effects, initially unexpected due to the lack of crystalline texture in these in-situ processed strands, appear to be due to a fibrous microstructure, connected with the details of the wire fabrication and MgB2 formation reactions. Scanning electron micrographs of in-situ-processed MgB2 monocore strands have revealed a fibrous microstructure. Grains (~100 nm) are randomly oriented, and there is no apparent local texture of the grains. However, this randomly oriented polycrystalline material has a fibrous texture at a larger length scale, with stringers of MgB2 (~ 60 {\mu}m long and ~5 {\mu}m in diameter) partially separated by elongated pores -- the spaces previously occupied by stringers of elemental Mg. This leads to an interpretation of the differences observed in transport and magnetically determined critical currents, in particular a large deviation between the two at higher fields, in terms of different transverse and longitudinal connectivities within the strand. The different values of connectivity also lead to different resistive transition widths, and thus irreversibility field values, as measured by transport and magnetic techniques. Finally, these considerations are seen to influence estimated pinning potentials for the strands.