Superconductivity at 23 K in Pt doped BaFe2As2 single crystals

TL;DR

This study reports the discovery of bulk superconductivity at 23 K in Pt-doped BaFe2As2 single crystals, demonstrating that substitution of Fe with Pt suppresses magnetic order and induces superconductivity with properties comparable to other transition-metal doped iron pnictides.

Contribution

First demonstration of superconductivity at 23 K in Pt-doped BaFe2As2, showing robust superconducting properties similar to other transition-metal substitutions.

Findings

Superconductivity at 23 K confirmed by magnetic and heat capacity measurements.

Superconducting properties comparable to other transition-metal-doped BaFe2As2.

Magnetic order suppressed and structural transition eliminated by Pt doping.

Abstract

We report superconductivity in single crystals of the new iron-pnictide system BaFe1.9Pt0.1As2 grown by a self-flux solution method and characterized via x-ray, transport, magnetic and thermodynamic measurements. The magnetic ordering associated with a structural transition at 140 K present in BaFe2As2 is completely suppressed by substitution of 5% Fe with Pt and superconductivity is induced at a critical temperature Tc=23 K. Full diamagnetic screening in the magnetic susceptibility and a jump in the specific heat at Tc confirm the bulk nature of the superconducting phase. All properties of the superconducting state including transition temperature Tc, the lower critical field Hc1=200 mT, upper critical field Hc2~65 T, and the slope dHc2/dT are comparable in value to the those found in other transition-metal-substituted BaFe2As2 series, indicating the robust nature of superconductivity induced by substitution of Group VIII elements.