Kondo screening in high-spin side-coupled two-impurity clusters

TL;DR

This paper investigates the Kondo screening phenomena in a high-spin two-impurity system with a side-coupled configuration, revealing how spin magnitude and exchange coupling influence multi-stage Kondo effects and thermodynamic properties.

Contribution

It generalizes the two-impurity Kondo model to high spins, analyzing the impact of spin sizes and exchange coupling on multi-stage Kondo screening.

Findings

Two-stage Kondo screening occurs for S_2 >= S_1.

Second Kondo temperature T_K^(2) scales as a power law for S_1 >= 1.

Thermodynamic properties depend on all three energy scales in high-spin cases.

Abstract

We study the system of two magnetic impurities described by a two-impurity Kondo model where only the first impurity couples directly to the conduction band, while the second impurity interacts with the first through Heisenberg exchange coupling in a "side-coupled" configuration. We consider various choices of the impurity spins (S_1<S_2, S_1=S_2, and S_1>S_2) and we contrast the regimes where the inter-impurity exchange coupling J is either lower or higher than the Kondo temperature T_K^(0) of the first impurity in the absence of the second. This model is a high-spin generalization of the two-impurity model for side-coupled double quantum dots which corresponds to the simplest S_1=S_2=1/2 case, where the moments are Kondo screened successively in two stages for J<T_K^(0) (the ``two-stage Kondo effect''). We show that the two-stage Kondo screening occurs generically for S_2 >= S_1. For S_1 >= 1, the second Kondo temperature T_K^(2) is not exponentially reduced, as for S_1 = 1/2, but is approximately a power-law function of the coupling J. Furthermore, for S_1 >=1 1 all three scales (T_K^(0), J, T_K^(2)) explicitly appear in the temperature-dependence of the thermodynamic properties. For S_1 > S_2, there is no second stage of screening for J<T_K^(0), however in the opposite limit J>T_K^(0) the Kondo screening of the effective spin S_1-S_2 is found.