Nonlinear magneto-optical resonances at D1 excitation of 85Rb and 87Rb in an extremely thin cell

TL;DR

This study investigates nonlinear magneto-optical resonances in an extremely thin cell for rubidium D1 transitions, revealing unique dependence on laser detuning and applying a detailed theoretical model to match experimental results.

Contribution

It extends the theoretical model of nonlinear magneto-optical resonances to extremely thin cells, accounting for their unique relaxation and Doppler effects, and compares with experimental data.

Findings

Resonance width and contrast depend strongly on laser detuning in the ETC.

Theoretical model successfully describes resonance shapes with modified parameters.

Agreement between experiment and theory is satisfactory, highlighting key physical processes.

Abstract

Nonlinear magneto-optical resonances have been measured in an extremely thin cell (ETC) for the D1 transition of rubidium in an atomic vapor of natural isotopic composition. All hyperfine transitions of both isotopes have been studied for a wide range of laser power densities, laser detunings, and ETC wall separations. Dark resonances in the laser induced fluorescence (LIF) were observed as expected when the ground state total angular momentum F_g was greater than or equal to the excited state total angular momentum F_e. Unlike the case of ordinary cells, the width and contrast of dark resonances formed in the ETC dramatically depended on the detuning of the laser from the exact atomic transition. A theoretical model based on the optical Bloch equations was applied to calculate the shapes of the resonance curves. The model averaged over the contributions from different atomic velocity groups, considered all neighboring hyperfine transitions, took into account the splitting and mixing of magnetic sublevels in an external magnetic field, and included a detailed treatment of the coherence properties of the laser radiation. Such a theoretical approach had successfully described nonlinear magneto-optical resonances in ordinary vapor cells. Although the values of certain model parameters in the ETC differed significantly from the case of ordinary cells, the same physical processes were used to model both cases. However, to describe the resonances in the ETC, key parameters such as the transit relaxation rate and Doppler width had to be modified in accordance with the ETC's unique features. Agreement between the measured and calculated resonance curves was satisfactory for the ETC, though not as good as in the case of ordinary cells.