Electromechanical instability in vibrating quantum dots with effectively negative charging energy

TL;DR

This paper investigates how strong electron-vibron coupling in quantum dots can lead to negative effective charging energy, causing instabilities and novel Coulomb blockade phenomena, which are stabilized by anharmonic effects.

Contribution

It introduces the concept of negative renormalized charging energy in vibrating quantum dots and analyzes the resulting Coulomb blockade features and their stabilization.

Findings

Negative effective charging energy can induce instabilities.

Anharmonic vibron energy regularizes the instability.

Double-well structure in charging energy affects Coulomb blockade.

Abstract

In quantum dots or molecules with vibrational degrees of freedom the electron-vibron coupling renormalizes the electronic charging energy. For sufficiently strong coupling, the renormalized charging energy can become negative. Here, we discuss an instability towards adding or removing an arbitrary number of electrons when the magnitude of the renormalized charging energy exceeds the single-particle level spacing. We show that the instability is regularized by the anharmonic contribution to the vibron energy. The resulting effective charging energy as a function of the electron number has a double-well structure causing a variety of novel features in the Coulomb blockade properties.