Resolution of the mystery of counter-intuitive photon correlations in far off-resonance emission from a quantum dot-cavity system

TL;DR

This paper explains why quantum dot-cavity systems show unexpected strong cavity emission off-resonance, revealing the mesoscopic effects that cause uncorrelated photon emissions despite originating from a single quantum dot.

Contribution

It provides the first comprehensive experimental and theoretical analysis of off-resonance photon correlations in quantum dot-cavity systems, highlighting the role of mesoscopic quantum dot properties.

Findings

Quantum dot confinement leads to a quasi-continuum of transitions.

Photon emissions at the cavity frequency are uncorrelated.

The model explains the counter-intuitive photon correlation measurements.

Abstract

Cavity quantum-electrodynamics experiments using an atom coupled to a single radiation-field mode have played a central role in testing foundations of quantum mechanics, thus motivating solid-state implementations using single quantum dots coupled to monolithic nano-cavities. In stark contrast to their atom based counterparts, the latter experiments revealed strong cavity emission, even when the quantum dot is far off resonance. Here we present experimental and theoretical results demonstrating that this effect arises from the mesoscopic nature of quantum dot confinement, ensuring the presence of a quasi-continuum of transitions between excited quantum dot states that are enhanced by the cavity mode. Our model fully explains photon correlation measurements demonstrating that photons emitted at the cavity frequency are essentially uncorrelated with each other even though they are generated by a single quantum dot.