Electronic structure of ferromagnetic semiconductor Ga1-xMnxAs probed by sub-gap magneto-optical spectroscopy

TL;DR

This study uses infrared magneto-optical spectroscopy to investigate the electronic structure of ferromagnetic semiconductor Ga1-xMnxAs, revealing insights into its band structure and spin-splitting effects related to ferromagnetism.

Contribution

It provides a semi-quantitative explanation of the infrared magneto-optical spectra based on the conventional disordered valence band theory with As p-orbital character.

Findings

Infrared magneto-optical effects relate directly to ferromagnetism.

The conventional valence band model accounts semi-quantitatively for the spectra.

Spin-splitting and spin-orbit coupling are key to understanding the electronic structure.

Abstract

We employ Faraday and Kerr effect spectroscopy in the infrared range to investigate the electronic structure of Ga1-xMnxAs near the Fermi energy. The band structure of this archetypical dilute-moment ferromagnetic semiconductor has been a matter of controversy, fueled partly by previous measurements of the unpolarized infrared absorption and their phenomenological impurity-band interpretation. The infrared magneto-optical effects we study arise directly from the spin-splitting of the carrier bands and their chiral asymmetry due to spin-orbit coupling. Unlike the unpolarized absorption, they are intimately related to ferromagnetism and their interpretation is much more microscopically constrained in terms of the orbital character of the relevant band states. We show that the conventional theory of the disordered valence band with dominant As p-orbital character and coupled by kinetic-exchange to Mn local moments accounts semi-quantitatively for the overall characteristics of the measured infrared magneto-optical spectra.