Orbitally induced string formation in the spin-orbital polarons

TL;DR

This paper investigates the formation of spin-orbital polarons in LaVO$_3$, revealing how holes couple to collective excitations and form stable quasiparticles influenced by both spin and orbital degrees of freedom.

Contribution

It derives a polaron Hamiltonian for a doped hole in LaVO$_3$ and demonstrates the formation of a stable spin-orbital polaron using the self-consistent Born approximation.

Findings

Identification of a stable spin-orbital polaron quasiparticle.

Hole confinement due to string-like potential from spin and orbital interactions.

Explanation of the role of spins and orbitals in polaron formation.

Abstract

We study the spectral function of a single hole doped into the (a,b) plane of the Mott insulator LaVO$_3$, with antiferromagnetic (AF) spin order of S=1 spins accompanied by alternating orbital (AO) order of active $\{d_{yz},d_{zx}\}$ orbitals. Starting from the respective t-J model, with spin-orbital superexchange and effective three-site hopping terms, we derive the polaron Hamiltonian and show that a hole couples simultaneously to the collective excitations of the AF/AO phase, magnons and orbitons. Next, we solve this polaron problem using the self-consistent Born approximation and find a stable quasiparticle solution -- a spin-orbital polaron. We show that the spin-orbital polaron resembles the orbital polaron found in $e_g$ systems, as e.g. in K$_2$CuF$_4$ or (to some extent) in LaMnO$_3$, and that the hole may be seen as confined in a string-like potential. However, the spins also play a crucial role in the formation of this polaron -- we explain how the orbital degrees of freedom: (i) confine the spin dynamics acting on the hole as the classical Ising spins, and (ii) generate the string potential which is of the joint spin-orbital character. Finally, we discuss the impact of the results presented here on the understanding of the phase diagrams of the lightly doped cubic vanadates.