Optical transition of the $^{229}$Th nucleus in a solid-state environment

TL;DR

This paper proposes a novel solid-state approach to measure the $^{229}$Th nuclear transition energy, potentially enabling highly precise optical frequency references and tighter constraints on fundamental constant variability.

Contribution

It introduces a method to drive the $^{229}$Th nuclear transition in a crystal environment, aiming for high precision measurements and improved fundamental physics constraints.

Findings

Potential to achieve frequency precision of 3×10^{-17} to 1×10^{-15} after 1 second

Systematic accuracy estimated at around 2×10^{-16}

Possible improvement of 100 to 1000 times in constraints on fundamental constants

Abstract

We describe a novel approach to directly measure the energy of the narrow, low-lying isomeric state in $^{229}$Th. Since nuclear transitions are far less sensitive to environmental conditions than atomic transitions, we argue that the $^{229}$Th optical nuclear transition may be driven inside a host crystal with a high transition Q. This technique might also allow for the construction of a solid-state optical frequency reference that surpasses the precision of current optical clocks, as well as improved limits on the variability of fundamental constants. Based on analysis of the crystal lattice environment, we argue that a precision of $3\times10^{-17}<\Delta f/f <1\times10^{-15}$ after 1 s of photon collection may be achieved with a systematic-limited accuracy of $\Delta f/f \sim 2 \times 10^{-16}$. Improvement by $10^2-10^3$ of the constraints on the variability of several important fundamental constants also appears possible.