Directional field-induced metallization of quasi-one-dimensional Li$_{0.9}$Mo$_6$O$_{17}$

TL;DR

This study reveals that applying a magnetic field to Li$_{0.9}$Mo$_6$O$_{17}$ can suppress a density-wave gap, induce a metallic state, and potentially lead to a new superconducting phase above 10 K.

Contribution

It demonstrates magnetic field-induced metallization and possible superconductivity in a highly anisotropic quasi-one-dimensional oxide, revealing new insights into field-tuned electronic phases.

Findings

Magnetic field induces negative magnetoresistance below 25 K.

Field suppresses density-wave gap, restoring metallicity.

Possible emergence of superconductivity above 10 K at high fields.

Abstract

We report a detailed magnetotransport study of the highly anisotropic quasi-one-dimensional oxide Li$_{0.9}$Mo$_6$O$_{17}$ whose in-chain electrical resistivity diverges below a temperature $T_{\rm min} \sim$ 25 K. For $T < T_{\rm min}$, a magnetic field applied parallel to the conducting chain induces a large negative magnetoresistance and ultimately, the recovery of a metallic state. We show evidence that this insulator/metal crossover is a consequence of field-induced suppression of a density-wave gap in a highly one-dimensional conductor. At the highest fields studied, there is evidence for the possible emergence of a novel superconducting state with an onset temperature $T_c >$ 10 K.