Production d'hydrog\`ene par oxydation catalytique partielle du m\'ethane Etude du m\'ecanisme r\'eactionnel

TL;DR

This study investigates the partial oxidation of methane using experimental and simulation methods to elucidate the reaction mechanism involving numerous homogeneous and surface reactions.

Contribution

It presents a detailed reaction mechanism for methane oxidation, validated through experimental data and simulations with Chemkin-Surface software.

Findings

Reaction mechanism includes 444 homogeneous reactions

Involves 33 surface reactions

Validated mechanism with experimental data

Abstract

The partial oxidation of methane was investigated using a self-stirred reactor under a wide range of operating conditions. The recation mechanism was determined by comparing ecperimental results with the results of simulations made using the Chemkin-Surface software. The proposed mechanism includes 444 homogeneous reactions and 33 surface reactions.